东亚夏季风对中国东部臭氧输送过程的影响研究
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中国气象局沈阳大气环境研究所

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东北地区大气臭氧时空分布特征和预报技术研究


Influence of Ease Asian Summer Monsoon on the ozone transport in east China
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Shenyang Institute of Atmospheric Environment, China Meteorological Administration

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    摘要:

    利用2015-2019年中国东部20个省份222个城市的地面O3观测数据和全球再分析风场数据,研究了中国东部地区O3的时空分布特征,以及在亚洲夏季风背景下污染上风方O3光化学输送对下风方O3浓度季节变化的影响。结果表明:中国东部地区O3浓度夏季高、冬季低,O3浓度按照东南、华东、东北、华北的顺序依次升高,位于中高纬度的华北、东北地区明显高于位于中低纬度的华东、华南地区。不同城市、不同季节O3浓度日变化形态具有较好的一致性,都表现为夜晚低、清晨逐渐升高、下午至黄昏达到最大的单周期变化形态,具有典型的光化学控制特征。春季,亚洲夏季风开始影响中国东部地区,华东、华北、东北地区为大范围的O3高值区;夏季,亚洲夏季风将O3及其前体物由纬度较低的华南、华东地区向纬度较高的华北、东北地区不断输送和累积,在夏季强紫外辐射作用下发生光化学反应,导致华北、东北地区夏季的O3污染。

    Abstract:

    We investigated the spatial-temporal ozone variations in eastern China by using surface ozone observation data from 222 cities of 20 provinces in eastern China and global reanalysis data for wind throughout 2015 and 2019, and evaluated the influence of the ozone photochemical transport from upwind directions to downwind directions in the background of Asian Summer Monsoon (ASM). It is shown that ozone levels over eastern China are high in winter, while low in summer, and increase in the order of southeast, east, northeast and north China. Ozone levels are significantly higher in north and northeast China located in mid-high latitudes than in east and south China located in mid-low latitudes. Diurnal variations of ozone levels exhibit similar single-period patterns that remain low at night, gradually rise in the early morning and peak during afternoon and twilight in various seasons over various cities, showing typical photochemical controlling characteristics. In spring, ASM starts to influence eastern China and cause a large region of enhanced ozone over east, north and northeast China. In summer, ASM persistently transports ozone and its precursors from south and east China to north and northeast China which react photochemically by solar UV radiation thus leads to summer ozone pollution in north and east China.

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  • 收稿日期:2020-07-06
  • 最后修改日期:2020-12-01
  • 录用日期:2021-01-18
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