银川市大气颗粒物物理化学特征研究Ⅰ:大气颗粒物浓度特征
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国家自然科学基金资助项目(40365003);南京气象学院科研基金资助项目(DQ08)


Physical and Chemical Characters of Atmospheric Particles in Yinchuan City, Part Ⅰ:Mass Concentration
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    摘要:

    根据大量的大气环境监测资料,系统分析了银川市市区、郊区以及市中各功能区(居民区、商业区、文教区、工业区、交通区、娱乐区)大气颗粒物的TSP(Total Suspended Particles)、PM10(粒径小于等于10μm的粒子)和PM2.5(粒径小于等于2.5μm的粒子)质量浓度的季节分布、日变化以及随高度的分布特征。结果表明:银川市背景大气TSP平均值为0.126~0.248mg·m-3,低于国家三级污染标准;银川市区TSP日平均浓度的年平均值为0.47~0.78mg·m-3,超过国家二级标准0.57~1.6倍,超标率高达61.3%~92.5%,日均最大值超标7.9倍;春夏秋冬4季中,以冬春两季日平均浓度最高,其原因是燃煤取暖和沙尘暴多发。各功能区中商业区、交通区、居民区的TSP较高,这显然与人为活动、机动车辆排放密切相关,TSP日变化均呈现出与人为活动相一致的规律性;TSP的空间分布表明城市高于郊区,规模大、人口密度高、商业网点密集的城区TSP较高。各粒径粒子的质量浓度随高度递减,PM10占TSP的比例却随高度增加,说明PM10随高度增加。地面呼吸带高度上PM10和PM2.5均较高,可能与低空排放源有关。春季风沙期是大气污染最为严重的季节。

    Abstract:

    The spatial and temporal distribution,diurnal variation and profile with height of atmospheric aerosol’s total suspended particles(TSP),PM10(particulate matter with a diameter equal to or less than 10 micrometers) and PM2.5(particulate matter with a diameter equal to or less than 2.5 micrometers) have been documented based on a large amount of environmental monitoring data at urban,suburb and different city functional areas,such as residential,commercial,cultural & educational,industrial,traffic,and park areas in Yinchuan.Results show that the averaged background atmospheric TSP is 0.126~0.248mg·m-3,less than that of National Pollutant Control Standard (NPCS) grade 3; the yearly averaged TSP is 0.47~0.78mg·m-3,1.57~2.6 times of NPCS grade 2;and the maximum daily average TSP is 7.9 times of NPCS grade 3.The probability of TSP greater than that of NPCS grade 3 is 61.3%~92.5%.The daily averaged TSP is greater in winter and spring than in summer and autumn,due to coal-burning for house heating in winter and sandstorms in spring.The TSP is greater in commercial,traffic and residential areas,it is closely related to the human activities and vehicle emissions.The diurnal variation of TSP accords with human activities.The TSP is much greater in urban area,especially in densely populated,heavily commercial activities and more urbanized areas.The segregated mass concentration decreases with height,whereas the ratio of PM10 in TSP increases with height,indicating that PM10 increases with height.PM10 and PM2.5 are large at about 2m above the ground surface,so it may be related to source emission near the ground.

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樊曙先,郑有飞,金国兴,陈世功,2004.银川市大气颗粒物物理化学特征研究Ⅰ:大气颗粒物浓度特征[J].大气科学学报,27(1):20-28. FAN Shu-xian, ZHENG You-fei, JIN Guo-xin, CHEN Shi-gong,2004. Physical and Chemical Characters of Atmospheric Particles in Yinchuan City, Part Ⅰ:Mass Concentration[J]. Trans Atmos Sci,27(1):20-28.

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  • 收稿日期:2002-12-16
  • 最后修改日期:2003-03-03
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